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Recycling that pesky Depleted Uranium and Nuclear Waste should be a very nice thing to have - apart from Radium, which is a subject on its own, I think that the nuclear fuel reprocessing could give a pretty straightforward crafting chain.
Like X depleted uranium + Y nuclear waste (let's imagine it as Plutonium) + Z refined carbon (graphite pellets would be prettier, Ronivan's Chemical Processing mod has Graphite in it IIRC) + W clay/ceramic for roleplaying the outer fuel vessel + Q oxygen/oxilite/fertilizer for voloxidation = K enriched uranium (let's imagine it as some MOX rods) + some kind of waste byproduct(s).
But ... I'm not very good at brainstorming recipes & co., after all - sorry!
Seems to work fine, at least for what I've seen by now!
i think that mod had some buildings that produced radium, but it was sadly removed some months ago...
i will look into your challenge collection mod, thanks for the hint :)